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A strategy for the immobilization of chiral 2,3‐bisaminocyclopropenium salt (pre‐catalyst) onto polystyrene and silica supports is presented together with a suitable procedure for the conversion into the corresponding cyclopropenimine superbase catalysts. The activity and recyclability of polystyrene‐ and silica‐supported cyclopropenimines were initially tested under batch conditions in a model Michael...
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