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In conventional adsorbate-adsorbent systems, for microdynamically indistinguishable species A and B, the total amount adsorbed is unaffected by intrinsic reactionsA->B. Under the conditions of molecular traffic control, i.e. for differing accommodation probabilities of the two species for different adsorbent segments, this simple rule collapses. As an example, mutually intersecting single-file...
Derouane and Gabelica postulated in the concept of 'molecular traffic control' (MTC) an enhancement of the effective conversion rate in catalytic reactions if the reactant and product molecules avoid each other by preferentially choosing different channel systems on their diffusion path into and out of the catalytic particles. As a main deficiency of this concept, so far no clear theoretical criteria...
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