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A new type of efficient CO2 absorbent with improved thermal stability is synthesized via self‐assembly between 2D inorganic nanosheets and two kinds of 0D inorganic nanoclusters. In these self‐assembled nanohybrids, the nanoclusters of CdO and Cr2O3 are commonly interstratified with layered titanate nanosheets, leading to the formation of highly microporous pillared structure with increased basicity...
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