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Visible‐light‐responsive photonic structures have been prepared in alcohol solvents by using silica‐modified PbS colloidal nanocrystal clusters (CNCs) as building blocks. Further modification of the PbS CNCs with a coating of silica allowed the dispersion of the particles into nonaqueous solutions. Repulsive electrostatic and solvation forces contribute to the self‐assembly of the PbS@SiO2 spheres...
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