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Photoelectrochemical and electrochemical reduction of CO2 into organic chemicals is promising for directly or indirectly transforming solar energy into chemical energy for further utilization. However, research on the electroactive species in these processes has been rather limited. In this work, we investigated possible electroactive species (CO2 or HCO3–) involved in the electrochemical reduction...
The silver-catalyzed, oxidative coupling of methane to C 2 hydrocarbons (OCM) is shown to be an extremely structure-sensitive reaction. Reaction-induced changes in the silver morphology lead to changes in the nature and extent of formation of various bulk and surface-terminating crystal structures. This, in turn, impacts the adsorption properties and diffusivity of oxygen in silver which is...
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