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The adsorption and oxidation of ortho-dichlorobenzene (o-DCB) over sulfated zirconia (SZ), Co–SZ, and Pd/Co–SZ were studied by means of in situ FTIR spectroscopy to determine the nature of surface intermediates formed on these catalysts. The results indicate that o-DCB adsorbs on Lewis acid sites, forming surface intermediates that are strongly held on the surface. These intermediates can be subsequently...
The oxidation of 1,2-dichlorobenzene (o-DCB) has been examined over Co–HMOR, Pd/Co–HMOR, Co–SZ and Pd/Co–SZ under dry and wet conditions. Under dry conditions, Pd/Co–SZ was the most active catalyst. However, in the presence of water Pd/Co–HMOR exhibits a significant activity while Pd/Co–SZ was not affected. Besides, by-product formation such as polychlorinated compounds decreased on both catalyst...
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