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Ein konformativ flexiblesC2‐symmetrisches chirales Iodosylaren, das mit Blick auf H‐Brücken‐ und sekundäre n‐σ*‐Wechselwirkungen gezielt entworfen wurde, katalysiert hocheffektiv die oxidative Kita‐Spirolactonisierung. Wie K. Ishihara et al. in der Zuschrift auf S. 2221 ff. beschreiben, wird mit dieser Katalyse eine höhere Enantioselektivität (bis 92 % ee) erreicht als in anderen durch chirale hypervalente...
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