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New types of one‐pot multi‐step enzymatic cascade transformation involving dynamic kinetic resolution to convert racemic substrates to chiral products in high ee and yield were developed. Unique cascade reactions of easily accessible racemic trans‐β‐methyl or α‐methyl epoxides to produce (S)‐2‐arylpropionic acids, (R)‐ and (S)‐2‐arylpropyl amines were demonstrated via styrene oxide isomerase (SOI)‐catalyzed...
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