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The front cover picture, provided by Seoksun Kim and Soon Hyeok Hong, illustrates the development of C–N and C–C bond formation reactions utilizing methanol as an environmentally benign C1 feedstock. Aminomethylation of phenol and methylation of naphthol were achieved via ruthenium‐catalyzed dehydrogenation of methanol without using any additional reagent. On the basis of various mechanistic studies,...
A reaction involving ortho‐aminomethylation of phenol was developed via ruthenium‐catalyzed dehydrogenation of methanol, an environmentally benign C1 building block, without the use of reactive reagents. The reaction was successfully applied to a range of substrates. When naphthol was employed instead of phenol, only methylation was observed. On the basis of various mechanistic studies, we propose...
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