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The reactions of methyl nitrite (CH 3 ONO) on O-covered Mo(110) were studied in order to determine whether methyl nitrite is a possible intermediate in CH 4 -assisted reduction of NO. Methyl nitrite decomposes to NO and methoxy (CH 3 O ads ) upon adsorption at low temperature. Most NO is evolved directly into the gas phase at 110 K, although a small fraction...
The coverage-dependent behavior of the vibrational spectra (high-resolution electron energy loss and infra-red reflectance-absorbance) of nitric oxide (NO) on a 0.75ML oxygen overlayer on Mo(110) is investigated. Intensity patterns in both sets of spectra are consistent with the conversion of surface nitrosyl species to dinitrosyls at higher coverages. Using sequentially dosed, isotopically mixed...
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