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The stereochemical activity of lone pairs (SCALP) in a cation favors the formation of acentric materials and can enhance the second‐harmonic‐generation (SHG) response and/or the birefringence. By introducing functional SbIII into sulfates, an anhydrous sulfate of Sb6O7(SO4)2 (1) is explored. Sb3+ cations are in seesaw configurations and in‐phase aligned in a 3D asymmetric dense structure. Compound...
By introducing the stereoactive lone pair cation of SbIII into sulfates, an anhydrous sulfate of Sb6O7(SO4)2 is achieved. Sb3+ cations are in seesaw configurations and in‐phase aligned in a three‐dimensional asymmetric dense structure. The material exhibits an enhanced phase‐matching second‐harmonic‐generation response, a moderate birefringence, a wide transparency window and considerable environmental...
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