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100keV H + scattering has been used to investigate the structure of the methylthiolate/Au(111) interface in the Au(111)(√3×√3)R30° phase. Adsorption of the thiolate onto the clean Au(111) surface leads to a large drop in the scattered ion yield due to the lifting of the clean surface ‘herring-bone’ reconstruction, but the thiolate-covered surface shows an ion yield higher than that of an unreconstructed...
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