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To achieve ecofriendly aerogels with high mechanics and fire resistance, naturally‐occurring pea starch was employed as the major substrate, and starch‐based composite aerogels were fabricated by freeze–drying method. The corresponding hydrogels were obtained through successive gelatinization/dissolution of pea starch and polyvinyl alcohol (PVA), formation of precursor hydrogels via cyclic freeze–thawing,...