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The full details of the original Ag‐catalyzed domino oxidative cyclization reactions of unprotected 2‐alkynylanilines with Oxone are described. The influences of several parameters including the substrate features, oxidant, reaction conditions, and catalyst on the reaction outcome were explored. A plausible mechanism is provided for the unusual silver‐catalyzed oxidative cyclization reactions of 2‐alkynylanilines...
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