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The photoexcitation of plasmonic nanoparticles has been shown to drive multistep, multicarrier transformations, such as the conversion of CO2 into hydrocarbons. But for such plasmon‐driven chemistry to be precisely understood and modeled, the critical photoinitiation step in the reaction cascade must be identified. We meet this goal by measuring H/D and 12C/13C kinetic isotope effects (KIEs) in plasmonic...
The photoexcitation of plasmonic nanoparticles has been shown to drive multistep, multicarrier transformations, such as the conversion of CO2 into hydrocarbons. But for such plasmon‐driven chemistry to be precisely understood and modeled, the critical photoinitiation step in the reaction cascade must be identified. We meet this goal by measuring H/D and 12C/13C kinetic isotope effects (KIEs) in plasmonic...
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