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An extended class of organic multi‐redox systems was derived from bicyclic(alkyl)amino carbenes (BICAACs). The highly‐conjugated system undergoes a total of 4 redox events spanning a 1.8 V redox range. These organic compounds exhibited four different stable redox states (dication, radical cation, neutral and radical anion), and all of them were characterized either by single crystal X‐ray study and/or...
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