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Solvent‐dependent, self‐discrimination of diamides is described. Mixing a solution of (R)‐1 a and (S)‐1 a, which are valine‐derived, bis(2‐hydroxyphenyl)diamide‐bearing, multiple hydrogen‐bonding modules, in dichloromethane immediately led to the formation of a thick suspension comprising a 1:1 heterochiral aggregate of 1 a. The solubility of heterochiral 1 a was substantially lower in halogenated...
Self‐discrimination ofS‐ and R‐valine‐derived bis(2‐hydroxyphenyl)diamides in an ensemble of eight structurally related molecules showcase their specific aggregation through the hydrogen‐bonding network of the bis(2‐hydroxyphenyl)diamide framework. For more details, see the Full Paper by M. Shibasaki, N. Kumagai et al. on page 5036 ff.
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