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Grand canonical Monte Carlo combined with molecular dynamics simulation methods are used to investigate the microstructure and oxygen permeability in hydrogels containing interpenetrating poly(bis(trimethylsilyloxy)methylsilylpropyl glycerol methacrylate) (PSiMA) and poly(2-methacryloyloxyethyl phosphorylcholine) (PMPC) networks at varying water contents. Water molecules are classified into hydrophilic-hydration...
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