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The synthesis of unprecedented benzimidazole‐fused thiazocines, thiazonines, and thiazecines having an exocyclic double bond is reported. The process proceeds through an 8‐, 9‐, or 10‐exo‐dig cyclocarbopalladation followed by reduction. The scope and limitations were established and showed the importance of the precursor structure for the success of the reaction. A competition between the exo‐dig...
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