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Self‐assembled vesicles with membrane‐embedded or adsorbed ruthenium polypyridine complexes were further functionalized by the adsorption of an [FeFe]‐hydrogenase subunit mimic to the membrane interface enhancing the photocatalytic hydrogen production in water under acidic conditions. The resulting two‐dimensional membrane assembly places the photosensitizer and hydrogen‐evolving diiron complex in...
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