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The complex formation of dibenzothiophene with chromium carbonyl complexes of the general formula L3Cr(CO)3 (L = Py, NH3, or CO) afforded η6-C12H8SCr(CO)3 (1). In the presence of tetramethylethylenediamine, complex 1 was selectively metallated with BuLi at position 4 of the coordinated ring to form η6-4-LiC12H8SCr(CO)3 (2). In decane, the tricarbonylchromium group is reversibly and intramolecularly...
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