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The bright yellow Schiff‐base complex Eu(TRENDSAL) (1) (TRENDSAL = N[CH2CH2N=CH(2‐OH‐3,5‐tBu2C6H2)]3) was prepared in 71 % yield by treatment of EuCl3·6H2O simultaneously with 3,5‐di‐tert‐butylsalicylicaldehyde and tris(2‐aminoethyl)amine in the presence of triethylamine. X‐ray crystal structure analyses of the solvates 1·DME (DME = 1,2‐dimethoxyethane) and 1·MeCN demonstrated the tight encapsulation...
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