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The multiple ways in which N2 can be coordinated to FeMo‐co, the Fe7MoS9C cluster at the active site of the enzyme nitrogenase, are catalogued and interpreted, in the context of other N2‐activating metal complexes. N2 bound to FeMo‐co is located in a unique gallery of surrounding hydrogen atoms, proposed to be a key factor in the conversion to NH3.
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