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Intrinsic hydrogen evolution reaction (HER) activity and the mechanism of antiperovskite Ni3In1‐xCuxN bulk cubic particles and multi‐crystalline nanoplates are thoroughly investigated. Stoichiometric Ni3In0.6Cu0.4N reaches the best HER performance, with an overpotential of 102 mV in its multi‐crystalline nanoplates obtained from the LDH‐derived method, and 143 mV in its bulk cubic particles from the...
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