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The weak electronic interaction at metal‐photocatalyst heterointerfaces often compromises solar‐to‐fuel performance. Here, a trifunctional Schottky junction, involving chemically stabilized ultrafine platinum nanoparticles (Pt NPs, ≈3 nm in diameter) on graphitic carbon nitride nanosheets (CNs) is proposed. The Pt–CN electronic interaction induces a 1.5% lattice compressive strain in Pt NPs and maintains...