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Hexamethyldisiloxane [HMDSO, (CH3)3‐SiOSi‐(CH3)3] is an important precursor for SiO2 formation during flame‐based silica material synthesis. As a result, HMDSO reactions in flame have been widely investigated experimentally, and many results have indicated that HMDSO decomposition reactions occur very early in this process. In this paper, quantum chemical calculations are performed to identify the...
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