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Layered van der Waals (vdW) crystals with intrinsic magnetic properties such as high Curie temperature (TC) and large perpendicular magnetic anisotropy (PMA) are key to the development and application of spintronic devices. The ferromagnetic vdW metal Fe3−xGeTe2 (FGT) has gained prominence recently due to its high TC (220 K) and strong PMA. Herein, a new metallic vdW ferromagnet, Fe5−xGe2Te2 or FG2T,...
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