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In this work, 1,5‐dihydro‐3,4‐dihydroxy‐2‐pyrrolone derivatives (XH2) and their anions (XH−) were designed and synthesized as the synthetic vitamin C analogs. The thermodynamic driving forces of the 8 possible elementary steps for XH2 to release 2 hydrogen atoms to become X in acetonitrile were determined using experimental methods. The mechanisms and the possible reaction intermediates of XH2 and...
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