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A photocleavable terpolymer hydrogel cross‐linked with o‐nitrobenzyl derivative cross‐linker is shown to be capable of self‐shaping without losing its physical integrity and robustness due to spontaneous asymmetric swelling of network caused by UV‐light‐induced gradient cleavage of chemical cross‐linkages. The continuum model and finite element method are used to elucidate the curling mechanism underlying...
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