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Linear molecules such as CO2 contain a positive π‐hole ring that surrounds C on the molecule's equator. Quantum calculations examine the question as to how many bases can simultaneously bind to this ring. Linear molecules examined are TO2, where T = C, Si, Ge, Sn; bases are NCH and NH3. CO2 engages in the weakest of the tetrel bonds, and can bind up to three NCH and two NH3. Unlike σ‐hole tetrel bonds,...
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