The digital reconstruction of microstructures is necessary for simulations in fields ranging from geology to electrochemistry, but the state‐of‐the‐art digital reconstruction techniques often compromise between resolution and field of view. It is challenging to retain detailed microstructure information in large‐scale reconstructions. This study investigates different aspects of the Yeong‐Torquato algorithm based on correlation functions to make it more efficient. We achieve this goal by reducing the computational complexity of the chord‐length distribution function and the two‐point correlation function, applying the random sphere‐packing method as the initial condition, and restricting potential voxel swaps to interfaces. In addition, a novel superposition parallel scheme is introduced to aid in searching for potential voxel swaps. The algorithm proposed is validated by comparing the pore‐size distributions of reconstructed 3D custom battery electrodes from a sample dataset obtained from transmission X‐ray microscopy. From a sample image with pixels, the code can reconstruct a structure in under 22 h and reconstruct a structure in 43 h with eight cores.