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Since the discovery of the hydroformylation (oxo‐synthesis or Roelen reaction) and the Reppe‐reaction, the transition metal‐catalyzed carbonylation reactions, providing versatile, facile, and even atom‐economic methods for the selective incorporation of C=O functionality to various skeletons, have gained tremendous importance in synthetic organic chemistry from laboratories to industrial applications...
Atroposelective synthesis of N‐N atropisomers is an emerging area but remains underexplored; in particular, the synthesis of N‐N benzimidazole atropisomers is still unprecedented. Herein, the first enantioselective synthesis of N‐N benzimidazole atropisomers via the palladium‐catalyzed de novo construction of benzimidazole skeleton is presented. With readily available palladium catalyst and biphosphine...
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