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Chain and ring [H2PEH2]n oligomers (E=B, Al; n=2–15) have been computationally studied at the B3LYP/def2‐TZVP level of theory. A strong tendency to cyclization was found for the chain Al–P oligomers with n>7, whereas analogous long B–P oligomers can exist as chain structures. Subsequent oligomerization enthalpies approach each other very closely for the ring and chain oligomers with an increase...
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