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Considering size effect and functionalized pore interaction dyes guests and MOFs hosts, 4‐aminonaphthalimide was successfully introduced into the pore of LnMOF for the first time and constructed 4‐ANA⊂LnMOF luminescent composites with excellent dual‐emission properties. A series of temperature‐dependent luminescence test results show that 4‐ANA⊂Gd4L3 can be used as a reversible ratiometric luminescent...
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