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Photoswitches and dyes in the liquid‐crystalline nematic phase have the potential for use in a wide range of applications. A large order parameter is desirable to maximize the change in properties induced by an external stimulus. A set of photochromic and nonphotochromic dyes were investigated for these applications. It was found that a bent‐shaped 7‐substituted dihydroazulene (DHA) photoswitch exhibited...
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