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We report the synthesis and X‐ray characterization of the N6‐benzyl‐N6‐methyladenine ligand (L) and three metal complexes, namely [Zn(HL)Cl3]·H2O (1), [Cd(HL)2Cl4] (2) and [H2L]2[Cd3(μ‐L)2(μ‐Cl)4Cl6]·3H2O (3). Complex 1 consists of the 7H‐adenine tautomer protonated at N3 and coordinated to a tetrahedral Zn(II) metal centre through N9. The octahedral Cd(II) in complex 2 is N9‐coordinated to two N6...
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