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Reaction of the Au–C N chelate [Au(bnpy)Cl2] with the full‐length zinc finger (ZnF; ZnCys3His) of HIV nucleocapsid protein NCp7 results in C–S aryl transfer from the AuIII organometallic species to a cysteine of the ZnF. The reaction is general and occurs even for finger 3 of the transcription factor Sp1, containing a ZnCys2His2 coordination sphere. This reaction is the first demonstration of group...
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