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Enzymes are valuable biocatalysts for asymmetric synthesis due to their exacting stereocontrol. Changing the selectivity of an existing catalyst for new applications is, however, challenging. Here we show that, in contrast, the stereoselectivity of an artificial enzyme created by design and directed evolution is readily tunable. We engineered a promiscuous artificial retro‐aldolase into four stereocomplementary...
Die Kompartimentierung chemischer Reaktionen ist ein grundlegendes Prinzip des Lebens und daher ein wichtiger Ausgangspunkt für Innovationen bei der Entwicklung neuer Ansätze in der Biokatalyse. Zur Implementierung von Biotransformationen in räumlich getrennten Kompartimenten werden daher Herstellungsmethoden benötigt, die die schnelle Produktion von in Flusssystemen einsetzbaren Biokatalysatoren...
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