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Determining whether a protein regulates its net electrostatic charge during electron transfer (ET) will deepen our mechanistic understanding of how polypeptides tune rates and free energies of ET (e.g., by affecting reorganization energy, and/or redox potential). Charge regulation during ET has never been measured for proteins because few tools exist to measure the net charge of a folded protein in...
Was passiert beim Transfer eines einzelnen Elektrons auf ein Protein? Ändert sich die Gesamtladung um eine Einheit oder spielt Ladungsregulierung eine wichtige Rolle? Durch die Beantwortung dieser Fragen könnten wir besser verstehen, wie Polypeptide die Reaktivität ihrer Redoxzentren anpassen. In ihrer Zuschrift auf S. 5462 zeigen B. F. Shaw et al., dass einige Metalloproteine während des Elektronentransfers...
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