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Tetra‐ortho‐substituted, heteroaryl and cyclic azobenzenes have emerged as three key strategies on morphology design of photoswitch to diversify controllability. Cyclic azobenzene is of particular utilization in photo‐energy conversion due to rigid and ring‐strain structure. Despite the well‐recognized diazocine, the photo‐switching properties of seven‐membered cyclic azobenzenes (diazepines) have...
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