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Reported herein is the first direct, metal‐catalyzed reductive functionalization of secondary amides to give functionalized amines and heterocycles. The method is shown to have exceptionally broad scope with respect to suitable nucleophiles, which cover both hard and soft C nucleophiles as well as a P nucleophile. The reaction exhibits good chemoselectivity and tolerates several sensitive functional...
Tribenzotriquinacene (TBTQ) is a bowl‐shaped molecule that has been widely used as a molecular building block in supramolecular and materials chemistry. Especially C3‐symmetric threefold‐substituted TBTQs are interesting for these purposes. Until now a general and selective synthetic approach to those C3‐symmetric products was lacking, mainly because the typically used electrophilic aromatic substitution...
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