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The use of secondary interactions between substrates and catalysts is a promising strategy to discover selective transition metal catalysts for atom‐economy C−H bond functionalization. The most powerful catalysts are found via trial‐and‐error screening due to the low association constants between the substrate and the catalyst in which small stereo‐electronic modifications within them can lead to...
Wie ein Enzym beschreibt am besten den supramolekularen Katalysator, über den Rafael Gramage‐Doria et al. in ihrem Forschungsartikel auf S. 18154 berichten. Die entfernt lokalisierten Zn⋅⋅⋅N‐Wechselwirkungen in einem Iridium‐Borylierungskatalysator sind für die einzigartige Selektivität und Reaktivität verantwortlich, die für die Funktionalisierung der C‐H‐Bindung von Pyridin beobachtet wurde. Das...
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