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Replacement of the carbon–carbon bonds of antiaromatic compounds with polar boron–nitrogen bonds often provides isoelectronic BN compounds with excellent thermodynamic stability and interesting photophysical properties. By this element‐substitution strategy, we synthesized a new B4N4‐heteropentalene derivative, 1, which is fully substituted with mesityl groups. Owing to kinetic protection by the sterically...
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