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Time‐domain synchrotron Mössbauer spectroscopy (SMS) based on the Mössbauer effect of 161Dy has been used to investigate the magnetic properties of a DyIII‐based single‐molecule magnet (SMM). The magnetic hyperfine field of [Dy(Cy3PO)2(H2O)5]Br3⋅2 (Cy3PO)⋅2 H2O⋅2 EtOH is with B0=582.3(5) T significantly larger than that of the free‐ion DyIII with a 6H15/2 ground state. This difference is attributed...
Einzelmolekülmagnete lassen sich mit 161Dy‐Zeitdomänen‐Mößbauer‐Spektroskopie analysieren. In ihrer Zuschrift auf S. 3482 beschreiben L. Scherthan, A. K. Powell, V. Schünemann und Mitarbeiter, wie anhand des 161Dy‐Kerns die magnetischen Eigenschaften Dy‐haltiger Verbindungen ermittelt werden können – direkt aus der Sicht des Lanthanoidions.
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