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A chemical vapor deposition strategy is leveraged to create a high‐density Fe single‐atom electrocatalyst, where 3.97 wt% Fe atoms are coordinated with square‐planar para‐positioned nitrogen and phosphorus atoms in a hierarchical carbon framework. The as‐crafted atomically dispersed Fe catalyst manifests an outstanding activity towards oxygen reduction reaction over the entire pH range, as demonstrated...
The past decade has witnessed the great potential of Fe‐based single‐atom electrocatalysis in catalyzing oxygen reduction reaction (ORR). However, it remains a grand challenge to substantially improve their intrinsic activity and long‐term stability in acidic electrolytes. Herein, we report a facile chemical vapor deposition strategy, by which high‐density Fe atoms (3.97 wt%) are coordinated with...
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