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We report interesting photomechanical behaviors of the dynamic molecular crystals of (E)‐2‐(2,4‐dichlorostyryl)benzo[d]oxazole (BOACl24). The photosalient effect of the rod‐like crystal based on a metal‐free olefin driven by photodimerization is observed. Moreover, the needle‐like crystals of BOACl24 exhibit a reversible bending away from a UV light source. The nanofibers curl easily under UV irradiation...
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