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DNAzymes are widely used as functional units for creating DNA‐based sensors and devices. Switching of DNAzyme activity by external stimuli is of increasing interest. Herein we report a CuII‐responsive DNAzyme rationally designed by incorporating one of the most stabilizing artificial metallo‐base pairs, a CuII‐mediated carboxyimidazole base pair (ImC‐CuII‐ImC), into a known RNA‐cleaving DNAzyme. Cleavage...
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