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A highly efficient copper‐catalyzed C−H/N−H cross dehydrogenative coupling between picolinamides and simple ethers was developed. The reaction was promoted by the chelation assistance of removable picolinyl group and exhibited excellent TON and TOF number. This method was applicable to both N‐aryl and alkyl picolinamides as well as various cyclic and acyclic ethers with good functional group compatibility...
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