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The lithium (Li) metal anode is confronted by severe interfacial issues that strongly hinder its practical deployment. The unstable interfaces directly induce unfavorable low cycling efficiency, dendritic Li deposition, and even strong safety concerns. An advanced artificial protective layer with single‐ion pathways holds great promise for enabling a spatially homogeneous ionic and electric field...
In article number 1808392, Jia‐Qi Huang and co‐workers develop a single‐ion‐conducting interface consisting of a dual‐layer architecture to protect lithium‐metal anodes. The artificial interface regulates a homogeneous ionic and electric field distribution and simultaneously brings a superior mechanical feature at the surface of the lithium‐metal anode, synergistically enabling a highly efficient...
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