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Despite the high theoretical capacity of lithium–sulfur (Li–S) batteries, a high cell‐level energy density and a long cycling life are barely achieved, mainly due to the large electrolyte‐to‐sulfur ratio, polysulfide (PS) shuttle causing the loss of active sulfur, and the formation of passivation layers on the Li anode. To raise the energy density, holding PS in the cathode has been the most popular...
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